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J. Appl. Phys. 59, 2619 (1986); http://dx.doi.org/10.1063/1.336989 (10 pages)

Picosecond study of near‐band‐gap nonlinearities in GaInAsP

M. N. Islam1, E. P. Ippen1, E. G. Burkhardt2, and T. J. Bridges2

1Department of Electrical Engineering and Computer Science and Research Laboratory of Electronics, Massachusetts Institute of Technology, Cambridge, Massachusetts 02139
2AT&T Bell Laboratories, Holmdel, New Jersey 07733

(Received 23 September 1985; accepted 7 January 1986)

From picosecond pump‐probe and forward degenerate four‐wave mixing (DFWM) experiments, we obtain the near‐band‐gap nonlinear absorption and refraction properties of GaInAsP for λ∼1.5 μm. Using a mode‐locked color center laser, the nonlinear signals are studied in room‐temperature samples as a function of time and wavelength for different pump energies and for materials with different band‐gap energies. Nonlinear absorption cross sections σeh as large as −5.7×1015 cm2 are obtained from the pump‐probe results, while effective nonlinear cross sections σeff as large as 7.8×1016 cm2 (corresponding to a steady state ‖χ(3)‖∼3.8×103 esu for a 20‐ns relaxation time) are measured in the DFWM experiments. The spectral behavior of the data shows that above the band gap, the nonlinearity is due both to band filling and screening of excitonic effects. However, the effectiveness of the screening diminishes within one or two plasma frequencies of the band edge.

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KEYWORDS and PACS

PACS

  • 42.65.Ky

    Frequency conversion; harmonic generation, including higher-order harmonic generation

  • 78.20.Ci

    Optical constants (including refractive index, complex dielectric constant, absorption, reflection and transmission coefficients, emissivity)

ARTICLE DATA

PUBLICATION DATA

ISSN

0021-8979 (print)  
1089-7550 (online)

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