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J. Appl. Phys. 111, 024307 (2012); http://dx.doi.org/10.1063/1.3677985 (8 pages)

Nanoscale magnetic structure and properties of solution-derived self-assembled La0.7Sr0.3MnO3 islands

J. Zabaleta1, M. Jaafar2, P. Abellán1, C. Montón1, O. Iglesias-Freire2, F. Sandiumenge1, C. A. Ramos3, R. D. Zysler3, T. Puig1, A. Asenjo2, N. Mestres1, and X. Obradors1

1 Institut de Ciència de Materials de Barcelona ICMAB-CSIC, Campus de la UAB, Bellaterra 08193 Barcelona, Spain
2 Instituto de Ciencia de Materiales de Madrid ICMM-CSIC, Sor Juana Inés de la Cruz 3, Cantoblanco 28049 Madrid, Spain
3 Centro Atómico Bariloche and Instituto Balseiro, Comisión Nacional de Energía Atómica and Universidad Nacional de Cuyo, South Carolina de Bariloche 8400, Argentina

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(Received 4 September 2011; accepted 16 December 2011; published online 24 January 2012)

Strain-induced self-assembled La0.7Sr0.3MnO3 nanoislands of lateral size 50−150 nm and height 10−40 nm have been grown on yttria-stabilized zirconia (001)-substrates from ultradiluted chemical solutions based on metal propionates. The nanoislands grow highly relaxed withstanding the epitaxial relation (001)LSMO[110]//(001)YSZ[010] and show bulk-like average magnetic properties in terms of Curie temperature and saturation magnetization. The interplay of the magnetocrystalline and shape anisotropy within the nanoisland ensemble results in an in-plane magnetic anisotropy with a magnetocrystalline constant K1(150  K) = -(5±1)  kJ/m3 and in-plane easy axis along the [110]-La0.7Sr0.3MnO3 direction as measured, for the first time, through ferromagnetic resonance experiments. Magnetic force microscopy studies reveal the correlation between nanoisland size and its magnetic domain structure in agreement with micromagnetic simulations. In particular, we have established the required geometric conditions for single domain, multidomain, and vortex configurations.

© 2012 American Institute of Physics

Article Outline

  1. INTRODUCTION
  2. EXPERIMENTAL DETAILS
    1. Nanostructure growth
    2. Morphological and structural characterization
    3. Magnetic properties measurements
  3. RESULTS AND DISCUSSION
  4. CONCLUSIONS

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KEYWORDS, PACS, and IPC

PACS

  • 75.75.Cd

    Fabrication of magnetic nanostructures

  • 61.46.-w

    Structure of nanoscale materials

  • 75.30.Gw

    Magnetic anisotropy

  • 75.30.Kz

    Magnetic phase boundaries (including classical and quantum magnetic transitions, metamagnetism, etc.)

  • 75.60.Ej

    Magnetization curves, hysteresis, Barkhausen and related effects

  • 81.16.Dn

    Self-assembly

International Patent Classification (IPC)

  • B82B1/00

    Nano-structures

  • B82B3/00

    Manufacture or treatment of nano-structures

  • H01F1/00

    Magnets or magnetic bodies characterised by the magnetic materials therefor; Selection of materials for their magnetic properties

ARTICLE DATA

PUBLICATION DATA

ISSN

0021-8979 (print)  
1089-7550 (online)

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